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I'm assuming that because the game is so new, the application simply doesn't allow the desktop composition to be toggled. Hopefully, someone has a way to change that.
https://www.sevenforums.com/software/249913-compatibility-settings-64-bit-applications.html
Unfortunately, it looks like there's no 32-bit version of Fallout 4. The store page says it requires 64-bit Windows, which usually means it's 64-bit software.
https://store.steampowered.com/app/377160/Fallout_4/
You are responding to a thread from 2015, champion.