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Kill sentinels which give nanites as you already know and refining the Pugneum they drop gives more nanites.
Find a planet with Curious Deposits, set up base kill them to get Runaway Mould, refine into nanites. (There are guides on this around as I believe it is the current best farm).
Find planet with gold and silver, set up gold and silver farm, refine gold and silver together into platinum, refine platinum into nanites.
If you have the money, sitting in 3 star systems in the station or outposts and sell the class A and S ships.
Just be aware that the last update changed part if the dynamics. I think it was only the inventory preservation with the free postsale swap that got nerfed tho so shouldn't affect the flip.
Single stage refining:
Platinum, Pungeum, Tainted Metal, Salvaged Data, Larval Core, or Hadal Core
Refining chain:
Residual Goop > Viscous Fluids > Living Slime > Runaway Mould > Nanites
Yes, 100% agree ... this is probably the quickest way to get large quantities of nanites.
To remember: refining of 9999 mould takes 20 minutes to get 1999 nanites. so you have to build some refiners as well (middle or large pref.).
in my case i use 3 refiners into my freighter, so i get like 6k nanites each turn... ofc i could build more refiners if i would...
so ... i farm mould min. 3 x 9999 ... port to the freighters refiners and run them ... go back to farm like 20 min or again min. 3 x 9999 ... repeat ... nothing easier than this
Larval cores
Hadal Cores
Savage tech modules
Tainted metal
Derelict freighters can yeild a fair amount of nanites in the form of the items above and directly from loot in the freighter. Many have slime to convert to nanites. They also have upgrades that can be sold for nanites the same as scrapping star ships.