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If you go to Library - Fallout 4 - and look at FO4's game description, Workshop, DLC etc.
Scroll down, you'll see all the DLC that you have bought and are avaliable for download. You'll see your DLC, checked. If you uncheck that, the DLC will be uninstalled. Rechecking that box will reinstall that specific DLC.
I don't know how that will effect your save files though, so uninstall and reinstall DLC with either more proper knowledge, or caution.
Good luck.