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Deleting them is the most common fix for the fatal error problem , you don't actually have to delete them, just move them to a different folder , then when the game starts it won't detect them and it will generate new default configurations.
This is the location of the config files C:\Users\YOURNAME\Documents\My Games\Borderlands 2\WillowGame\Config
I've had the fatal error before , it seems to pop up randomly so I'm not sure what caused it for me , sometimes deleting just those two files isn't enough , so a quick thing you could do instead is to cut everything in the config folder and paste it in a new folder on your desktop , try to run the game , if it works that's the fix , if it still doesn't work you can put the config files back.
If deleting them didn't work you will need to put in a little more effort , you can try to read the error text to see if it mentions anything specific , DLC , DLL , MIssing File etc etc, or you can copy and paste the text and try googling it for the answer.
These fatal errors have been pretty common , you can even try searching these steam topics for "fatal error" and see a bunch of them recently popped up.
Please mark Radiowavehero answer as correct, that way it will get pinned at the top and will be easier to find when others look for a solution to this problem