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Alternatively you can seek help from a doctor for a small free. Or if you've fought some Super Mutants, be sure to loot their mutated hounds for their meat. If cooked it will slightly reduce your radiation poisoning.
Finally - You can craft Radaway by yourself with a chemical laboratory if you have the right ingredients (You can see which ones you need by looking at the recipe there)
Um incidentally, I also put on anti rad gear when I go wandering in water or if it rains or there are ghouls about. the gas masks, or sack hoods and stuff actually do help and reduce the rate of radiation received.
Anyway I've used only 2 rad aways so far, but used several in making different chems and have made them just to sell or stockpile inc ase I need them later.