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Kill them in their initial vault, and add some new enemies to random encounters, and at least one quest from the Castle later on, dealing with them that way.
Oh... I see. Did you finish the mass somethig quest (that they mention on mod page) or just visited institute for the first time? And did it allow you to rescue the leaders inside valut 111 despite being blocked later?
It let me rescue them, and the quest line plays out, until it gets to it's version of The Molecular Level, at which point, the chain gets stuck, because you've already been inside the Institute. So you can't finish the quest chain associated with the mod.
I imagine you could console command your way through that initial obstacle, but that comes with it's own set of risks, and so it's easier to just start a new game, and play it that way. You may want to anyway, because there are various choices to be made, that can change outcomes, which means it's something that you can't play just once to see everything anyway, w/out creating a lot of hard saves along critical paths, anyway.
Dammit, I guess I would need to start over.
Which means I will be level 1.
Well I wanted to try the game on PS5 anyway.
Thanks for your help :)