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http://fallout.wikia.com/wiki/Enclave#The_Vault_Experiment
I always assumed Vault-Tec and the Enclave wanted the Nuclear War, they saw the world had reached a point of unsustainable "Dead Weight" and needed to shed what they deemed were "Undesirables"
Part of weeding out, and eventually "Improving" human society was testing various stressors and situations through the Vault-Tec program. They needed to learn, in proper, controlled environments, what the limits of human psychology and physiology were, in order to create a more effecient human society.
What most people don't realize is that much of the games Vault-Tec Expirement theme is inspired in part by expiriments conducted on both civilians and Soldiers by the US government in the 1940's, 50's, 60's and 70's regarding radiation exposure, viral/Chemical warfare, individual isolation, and other mental and physical and even social situations.
Millitary ones range from the Fev vault,the musician vault and the gas vault (just to name a few)
Social experiments were vault 101, Vault Gary,and any of the control vaults
Giggles are vault 69,68,& vault 72(again to name a few)
The Enclave ran Vault Tec. The reasons are explained on the wiki.
http://fallout.wikia.com/wiki/Enclave#The_Vault_Experiment
At the core of survival is chaos theory. In essence the mad schemes all come down to the concept that out of random adversity, evolution occurs. Causing mankind to become more able to survive and thrive as a species. With some Vaults serving more specific diabolical purposes and individual agendas.
So in a sense, a type of forced Darwinism.