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Are you just asking which armour looks the best? I think that's just down to your personal taste.
EDIT: In general, it depends what you're after. I think marine tactical armour is the heaviest and has the highest rating (I'm not sure about Nuke World armour, though), but it doesn't generally have a chance to produce legendary effects, just the set ones you buy and the non-legendary ones all those zealots wear.
the strongest non-pa armour otoh afaik is the assault marine armour from far harbour.
If you don't care about legendary effects you can make a full set metal armor (heavy) with the armor fabric in contraptions dlc. It looks amazing and has the best ballistic resistance. Also mod it with ultra-light for a minimal weight and you're good to go.
I think only the marine armor from FH beats the heavy metal but I'm not sure
With a full set metal (polished) and ballistic weave you can get over 300 DR , that makes you almost immortal
here you can see many interesting things:
http://fallout.wikia.com/wiki/Fallout_4_armor_and_clothing
Like the mechanist armor, Old Longfellow outfit, any Atom's child robes (they look badass), courser outfit
If modded identically, the Operator Heavy Chest Piece has 55/55/ DR/ER and weighs the same as the Disciples chest piece.
probably one of the mods I'm using, ballistic weave you can use on things like the bathrobe (because reasons) but not silver shroud armour.