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This is the build I run using pimpernels:
http://bl2skills.com/assassin.html#505051045150455105015050500000
I don't grab execute because it is situational. There are very few instances in which it is actually useful, but even then it's unnecessary. I prefer to max f0ll0wthr0ugh for the speed and dps boost.
I don't grab ir0n hand because it is a useless skill in general. I adds a negligible amount of melee damage due to where it lies in the damage formula (it's also additive damage), and the extra health is a nuisance for health gate (remember that you are the squishiest character).
Tw0 fang is not your friend for critical ascension, even when using the lyuda. It's not good to take it as a sniper Zer0. It will usually cause you to miss upon proccing. Better to stick those two points in fearless.
Precisi0n is only marginally useful, even with a lyuda. It will make the 3-pellet split a bit tighter; however those points could be used elsewhere. You can also manage the split by finding hte lyuda's sweet spot and shoot from that distance.
I don't take vel0city because it messes with the pimpernel's spread. The more points you have in vel0city, the more you will have to offset your aim. However you can still take vel0city and adjust your aim accordingly (I simply don't like to, but you can give up kill c0nfirmed for it very easily). I also messes with the distance that the lyuda pellet splits into 3, so you will have to account for it when shooting (the idea is to get the bullet to just spread before hitting the critical hit spot)
If you want to use the lyuda this will serve you much better:
http://bl2skills.com/assassin.html#505121515150455105015050500000
The lyuda is much more useful for critical ascension. The pimpernel is not good for critical ascension, but it's much powerful on its own and is better for ammo consumption.
I will almost always switch to lyudas anyways for raid bosses as it is usually the better option in that case. I just prefer the pimpernel for mobbing.
General tips: Always stay mobile, and use deception to exploit b0re, kunai, and ambush whenever possible. Aiming down you sights and triggering deception causes you to skip the animation and enter deception instantly (can save your life). Zer0 also throws his decoy at a 45 degree angle, so jump up to the side and turning enough before triggering deception will place the decoy directly behind you (can also save your life).
Sniper stockpile relic helps (I use this for mobbing, but will switch to a bone of the ancients during raid boss fights). I would also not recommend a bee shield for mobbing, but an antagonist instead.
Can't remember other stuff off the top of my head right now. Hope this helps.