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Your issue isn't a problem with the amount of bits.
As far as reinstalling Steam goes. I'd copy the game folders outside of Steam, reinstall Steam, copy the game folders back. When you go to install a game, it'll detect previously existing files and skip downloading and go right to verification and finishing.
This is probably your problem of Steam having issues launching at first.
The Steamapps, and the Userdata. Rename them steamapps_old and Userdata_old.
Cut them and place into a new folder outside of Steam folder name that folder you identify with like my steam stuff.
.
Then delete everything else restart Steam and it reinstalls clean
replace the 2 folders from your backup.
Here's the Steam clien download page but you dont really need that.
https://store.steampowered.com/about/
I see, that solution makes sense, I know that all game info is in steamapps so what is stored inside userdata that is important and is always stored locally? On the meantime, is there any other folder that might contain local only information that I should backup as well?
https://help.steampowered.com/en/faqs/view/4578-18A7-C819-8620
Because everything has to be set up properly to hopefully avoid problems. And in this case, I can't be sure that is the issue, but it could be, due to the drive being slow to start perhaps or security software having an issue with the drive, perhaps.
https://help.steampowered.com/en/faqs/view/1F39-DCB4-FF28-5748
There are a few possibilities, but none of them have anything to do with the bitage of your OS, as explained by the good Snakub.
Fortunately, there is an easy test you can do to rule several things out :
Boot your PC into safe mode with networking enabled in the boot options. It has to be WITH networking. Then only run Steam in this boot. As long as there are no issues with the drive connecting in this boot, there should be no issues with Steam running in this boot.
For example, if software conflicts with Steam running in a normal boot, that software will not do this in safe mode with networking, because it does not start automatically in this boot.