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Because just moving the files will not help, they have registry entries and a path that Steam follows to find them. Make sure that your steam properties for each game has the correct path to locate the game.
You might need to add new exceptions to such programs, since you changed the path where they are now installed.
This thread is old, so some things have changed in the Steam client but the client has a way to move games that you have installed, when you have more than one library.
If you manually moved the game files, that's also a problem, as there is an .acf file in steamapps that also had to be moved properly. (EDIT...Although to be fair, this would not allow you to verify the files as you said you did, as Steam would not be able to see them)
If not, Steam cannot even see that you have the game installed.
So it really matters what exactly you moved and how you did it.
That could possibly be the issue. See here :
https://help.steampowered.com/en/faqs/view/1F39-DCB4-FF28-5748