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Glitching Armory I'd say is the best since Pearlescent weapons can be found in the crimson lance chests, while easily being do able solo.
Soloing Crawmerax is pretty slow unless you modded in a one hit kill weapon, then it'd be the best.
I haven't opened the Gold key chests enough to tell if Pearlescent are available.
After that, the armory is your best bet IMO.
Getting the loot midgets is worth it, but isn't that a one time thing? I don't know how that works, because I was last there like 5 years ago? I didn't finish the DLCs yet this time.