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The top tier crafting materials mainly drop from the Ancient Path. Note that sometimes (as rewards for finishing an encounter) you will get "one of this now" with the idea that "a bit later you will be able to get more", so that's likely where you got it from. Alternatively, Bandit Kawas will drop stuff from about "one tier higher" than you can normally get, so they would likely be your best shot before doing Ancient Path.
For some more details, check out:
https://steamcommunity.com/app/699170/discussions/0/3247565033764140328/
https://steamcommunity.com/app/699170/discussions/0/1649918058730348460/
https://steamcommunity.com/app/699170/discussions/0/1648791520837645889/
My apologies, I got confused by what you were saying.
As for [Quality Thread], I see that it's a more "mid-game" resource, so trying in Crossroads is likely not your best bet. https://ibb.co/C9b2rz5 screenshot for people's reference in terms of "this is what it's used for", and why I was saying "mid-game" resource.
As I am not at my gaming PC right now, I cannot check specifically, but I would recommend following the details which I had put in the third of those threads I linked above in terms of "seeing in the game files where X drops".
I wish I could give you more guidance offhand, but my gut feeling says "if it's a mid-game material, try mid-game areas".