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There is also a possible way by hunting tempered barroth and tempered radobaan before so the quest will pop up, though it's not really proven.
I got the quest. I'll explain what I learned in case someone else who finds this topic is confused like I was.
They have to be 5 different types of monster. It's not enough to just kill a raithian 5 times like I did, they have to be unique creatures. This means one raithian, one barroth etc etc...
Even if you kill something considered Threat level 1 (ie, the two threat level 1 bazelguese you fight after beating xeno'jiiva) unless they are present on the list below they will not count towards the quest. Only these tempered creatures do:
-Pukei Pukei
-Tobi Kadachi
-Anjanath
-Barroth
-Jyuratdodus
-Rathian
-Paolumu
-Radobaan
I creatures I killed specifically were the Tobi, Anjanath, Rathian, Barroth and Radobaan. I'd say you're probably right about the Radobaan and Barroth. If someone else is looking to do the quest I'd make sure you hunt them just to be sure.
All you really need is one investigation, and you can unlock all the others from picking up tracks from said creature. I ended up with over 20 unique tempered investigations for pretty much every monster I needed by just following a rathian around for a bit. It's much faster than going and wandering around in an exhibition looking for the odd track which doesn't even give anything.