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As for properly removing the files, the "delete" button isn't going to mess up anything. What you need to be concerned about is whether the registry information got removed as that can sometimes seriously interfere with reinstalling later. I'd recommend looking at cruinne's troubleshooting guide for the step-by-step on how to do that, but you could resort to a registry cleaner of some sort and get the same effect.
https://steamcommunity.com/sharedfiles/filedetails/?id=279488894