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The chapters can be completed on normal or harder, so it's usually unlocked after beating the game on normal, hard and NSIC, since you have to beat them anyway to get Bazillions, Pillow Talk, Bracelet of Time and Climax Brace (you will get more than half of the chapters needed that way).
Anyway, the shortest chapter would be The Lumen Sage (especially if you have the Bracelet of Time, which will let you do massive amounts of damage and skip the QTEs in each phase).
If you get bored and want other short chapters, The Vestibule and the Cardinal Virtues chapters are also fast to beat. The Broken Sky also lets you skip a lot of verses but it's not really worth it.
But yeah, unlocking the Sai Fung with each character is the most boring one, so unless you really want to use the Sai Fung early on, I would just wait until you get other unlockables and pure platinums so you unlock it naturally that way.
With Bayonetta at least unlocking Jeanne and the Bracelet of Time usually means completing the game on normal twice, adding Hard and NSIC leaves you with around 30 chapters to complete, so I'd say it's less boring.
With Jeanne and Zero you usually know all the optional stuff like alfheims, beating the game under three hours and all that so you are left with more chapters to complete, so I wouldn't try unlocking it for Jeanne right after doing it for Bayonetta.
The Lumen Sage takes 3 to 4 minutes, so that would take around 5 hours after completing the game once.