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Here's a chart on how each type of metal you are refining will raise each "batch" of coolant for different liquids (chart is towards the bottom; you will need to expand the link to see chart):
https://oxygennotincluded.gamepedia.com/Metal_Refinery
otherwise yeah using it for smelters first is a good way to go.
I wonder what would be better.. Pump all your air through the cold water, or pump the cold water through the warm air... hmmm. Lol
if you didnt mind the slight decor penalty, you could run radiant pipes and run a water loop for a specific room though. but if you cant purge those pipes because of an overflow of your cooling system your stuck with that room becoming cold. both work but depending on your intent of use one is better than the other. atleast early on. later you'll be using the aqua tuner and HVAC for those kinds of things.
Fully depends on the heat within your base, or if you even need cooling depending on temp of map. Just an idea.
Use the water to cooldown the oxygen created, into a sieve, into the electrolyser(s). Exces water will also be warm enough to be used in your base.
This way your spom is self sustained and self cooled at no additional cost beside the first time setting/builing it up.
With other words, free cold breathable clean air!