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Best way is to hang around dolmens, or go after world bosses with groups. They drop a bunch of gems.
That said, since the One Tamriel update, there are only grand soul gems in the game (you can get some small gems lying around but they are mostly relics that were forgotten by the devs), because of the unique scaling mechanics of the update any other soul sem would be non adequate (every monster is lv 50 cp160 in the game, so any gem that is not a grand gem doesn't work anymore).