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After unlocking and completing mission 45, players will then need to complete all story missions up but not including 46, finish every highlighted (with yellow) Side Ops mission, and upgrade their Mother Base to nearly max potential in order to unlock Mission 46. Once that’s done, it’s time to go get the infinity bandana.
Upon completion of Mission 46 players will earn the Star of Bethlehem, another unique item essential to the infinity bandana’s development. Once acquired, players can use the Star of Bethlehem with a Research and Development level of 48 and 1,000,000 GMP to develop the infinity bandana. Again, wait the development time and infinite ammo will be yours.
Source:
https://gamerant.com/metal-gear-solid-5-bandana-guide-128/
Maximum bond with quite, watching huey's cutscene, using anything but the buttlefly emblem in your FOB.