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Tainted Brain Matter is a crafting material.
It can be looted from Aetherials and Aether Corruption Heroes and Bosses.
Trove?
That was probably why you couldn't get any from the Warden.
The sealed chests you have to dynamite open.
I'm sorry; I realised I should have elaborated after posting my comment, but was too lazy to edit it.
I meant, where is there a trove in Deadman's Gultch? I'm only aware of the small side area halfway between where the aether begins and the locked gate, though I wasn't even aware of that until I read your comment and went back to explore. Is the trove in the area behind that gate? I looked it up on the wiki, and it appears to stay locked until some point in Act 4.
It seems the OP is around the same level of progress as I am, so the gate remains locked. Also, aren't those chests one-time only, making them irrelevant for farming?
Most (maybe all?) troves have one of several locations they can spawn in, so they're not always in the same place. There is a guide with all locations in the guides section here on Steam.
Ahhh... Okay, thanks.
[edit] Also, thanks to Old Iron Johnson for mentioning Deadman's Gultch. Cracked a beer and spent like half-an-hour collecting some good materials. That's a nice quick spot for that.
[edit ps] Got two tainted brain matters, by the way, Alien.
Mountain deeps or whatever Ikrix's hideout is called, either in two spots along the left side of the map, or near the center between the two large gaps in the level.