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You also need to completely exit out of Steam before opening aliasIsolationInjectorGui.exe, otherwise the mod doesn't work.
(Strangely, the mention of needing to exit Steam is only called out on the GitHub README.txt, not the README.txt included with the release download...)
https://github.com/aliasIsolation/aliasIsolation
Make sure those settings are active and Steam is completely exited (not minimized) before running aliasIsolationInjectorGui.exe, then you just click "Launch Alien: Isolation" and it should work. You can tweak the sharpening and chromatic aberration while the game is running. There will be an obvious "Alias Isolation" icon at the top left corner of loading screens if it's working.
I'm using version 1.0.6 of the mod, which appears to be the most recent.
https://github.com/aliasIsolation/aliasIsolation/releases/tag/v1.0.6
https://github.com/RyanJGray/aliasIsolation
The "latest" legally obtained steam version of the game is about 10 years old.
PJ is correct.
The most modern version of the TAA mod is April 2024, which works on windows 10 (up to date). I check it every month or so and update my specific thread about the matter, which is here.
People are pushing the 8 year old version of the mod, for no sensible reason, other than perhaps they are comfortable with it and can therefore recommend it easily as they can also support the people who need help with it.
My thread about RyanJGray's April 2024 version is here:
https://steamcommunity.com/app/214490/discussions/0/4289188745217202131/
(I checked last week and it still works for me - win 10 up to date, i5-4690, nvidia 1660super)
Obviously, I should add that both versions of the T(AA) are offsite, therefore not checked by steam, other than perhaps steam moderation allowing the links to be posted here.