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It's going to make you run an install command from terminal, then just like with those old windows games, you'll likely have to jump through some hoops due to compatibility and it being so old.
Can you share this file contents? That way we'll see what it tries to do.
Also, it would be useful if you posted a listing of that ISO files and folders. You said you extracted it, so you can then go to that place in terminal/console, run tree command there, and post the output to some pastebin.
You will need to install some libraries (the Loki compatibility libraries) which will require you to take the Steam Deck filesystems out of read-only / immutable mode; and you'll need to set an environment path variable which...
Honestly, would be much less cumbersome to get the Windows SimCity 3000 Unlimited version DRM free on GOG and use the Heroic Games Launcher...
https://www.gog.com/en/game/simcity_3000
https://heroicgameslauncher.com/
you have this, right? https://archive.org/details/sim-city-3000-unlimited
Ironically, it's a lot easier to install old Windows software into the deck than old linux software. Buy the windows version thru GOG and run it thru Heroic games launcher, or download a windows iso and run it thru Bottles.