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You can try and farm cap stashes but that just seems like a time waster like farming the treasure hunting maps.
Second way, which relies on certain dailies being available but some players cannot do this as their daily quests may or may not be bugged. The Hemlock holmes golf course daily can be repeated for me. Turn in, leave zone, come back and turn in again. something like 60 caps and 3 scrip each time. Just have to farm up some radstag meat and tatos. The other daily is Chloe in Berkeley Springs. She can be repeated for me too. Do her quest, leave zone, return and it should say "Investigate Berkeley Springs" again, talk to her and she wont open up a dialogue box, which is ok. Now quit out and hope servers. Talk to her again and she will give the quest again. Its 90 caps and 7 scrip each time. Or you can do daily ops over and over again. Its either like 50-500 caps or 10-50 scrip each run (under 8 minutes not sure if that effects the caps/scrips rewards, I just stay under it everytime to be sure). Its a grind but if you got the time and the need for caps/scrip.
Riding Shotgun pays an extra 100 caps if you do the bonus.
Most mini-events marked on the map pay 20-30 caps each.
generally 16-20 caps