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Two things to try: ensure your registry is clean of game keys you're not using (esp. important if you've had Sims 3 previously installed then uninstalled it).
Second: factory reset. Go into your computer's Documents directory, then into the Electronic Arts folder. Inside there, rename the "The Sims 3" folder to somethinge else (like, "Old Sims 3"), and see if the game will start.