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Shut Steam down completely.
Copy your C:/Program Files (x86)/Steam/steamapps to E:/Steam/steamapps.
Once completed, relaunch Steam and let it find the games that were originally on the C: drive. Steam may run a verification on the files and "update" them but it shouldn't think to download the entire game again.
When you've verified that Steam can see them on E:, you can delete the ../steamapps folder from the C: drive to relieve some space.
Alternately, you can add the C:/Program Files (x86)/Steam/ as a separate Steam Library folder and just use Steam's internal move folder function.
edit: made some clarifications to storage locations and details.