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Exit Steam Client.
Delete the new folder, rename the old one again.
I've done it this way for years and it has always worked as simple as this.
In Windows OS however (in Control Panel > Power Options) you will want to select High Performance power profile > then Edit it > under HDD make the sleep timer very lengthy.
Otherwise if the secondary drive goes to sleep; and you launch Steam, those games might not show as installed; due to Steam not able to look at that drive when asleep/low-power mode.
If Steam does have an issue writing to the Steam Library Folder Location on your External HDD when change system; exit Steam Client, go to that Steam folder on external HDD, right click it, click Properties, click the Security tab; and then select Users and also any UserNames for said system; edit the security for those to have "Full Control"