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https://www.nexusmods.com/skyrimspecialedition/mods/120570
https://www.nexusmods.com/skyrimspecialedition/mods/133266
Guard dialogue overhaul and/or extended guard dialogue so guards don't ask you about your stolen sweetrolls every time you pass them or brag to you about their marriage (Arrow in the knee)
https://www.nexusmods.com/skyrimspecialedition/mods/22075
https://www.nexusmods.com/skyrimspecialedition/mods/106523?tab=description
Relationship dialogue overhaul
https://www.nexusmods.com/skyrimspecialedition/mods/1187
Interesting NPCS, adds tons of new and interesting NPCs with... Most of them lore friendly.
https://www.nexusmods.com/skyrimspecialedition/mods/29194
More to say, gives you more dialogue options with NPC's, although it just shuffles through their vanilla lines.
https://www.nexusmods.com/skyrimspecialedition/mods/22622
Ai overhaul makes your NPCs sometimes act like a real person would.
https://www.nexusmods.com/skyrimspecialedition/mods/21654
Someone already mentioned chatty NPCs and followers, that ones good too.
You could also look into follower mods, there's a lot of great ones out there like Lucien for example.
I would also suggest looking up Jayserpa, they have a bunch of great mods that add lines to existing npcs and overhauls some quests In fact I would suggest looking through all of his mods, everything he does screams immersion.
If questing is your thirst, then you should explore quest heavy DLC-sized mods such as:
* Enderal (needs a new playthrough, doesn't work well with followers, but it is awesome game in its own right, with tons of content)
* Vigilant (it's part of a trilogy by Vicn; Vigilant is finshed, Glenmoril and Unslaad almost)
* Legacy of the Dragonborn (excellent player home & collector's museum, but also great quest)
* The Forgotten City (so good it even won a national Writer's Guild award for its stellar script, and it has been converted into a standalone video game)
More recommendations on quest mods can be found on these threads:
https://www.reddit.com/r/skyrimmods/comments/14xqtct/quest_mods_worth_playing_in_2023/
https://www.reddit.com/r/skyrimmods/comments/qes0bj/skyrim_sse_quest_mods_masterlist_2021/
It might also be an eye-opener not to roleplay as the Dragonborn. Use an alternate start mod, and start questing and adventuring in your own unique ways:
https://www.reddit.com/r/skyrimmods/comments/1h82hor/what_is_the_appeal_of_a_nondragonborn_playthrough/
https://www.reddit.com/r/skyrimmods/comments/18ln5th/good_alternate_start_mods/
Off the top of my head (actually a little list from one of my personal notes about quest mods, LOL):
Enderal: Forgotten Stories, Wyrmstooth, Undeath, Glamoril - The Maze of Labyrinthian, Falskaar, The Wheels Of Lull, Moon And Star, Vigilant, Uslaad, Forgotten Dungeons, Carved Brink, Helgen Reborn, Project AHO, Beyond Reach, Interesting NPCs, Beyond Skyrim: Bruma, Legacy of the Dragonborn, The Forgotten City, Shezzarine: The Fate of Tamriel, Moonpath to Elsweyr, Fight Against the Thalmor, Into the Depths, Psijic Realm, Summerset Isle, Maids II – Deception (NSFW), The Tools of Kagrenac, The Gray Cowl of Nocturnal, Salem, Missives, Here There Be Monsters (fight mega monsters!), The Sinister Seven (reverse quest; here YOU are the quest target as you are marked for death/assassination, and chased around Skyrim by 7 progressively challenging enemy bosses).
Bigger (excellent and exhaustive) list here:
https://www.reddit.com/r/skyrimmods/comments/qes0bj/skyrim_sse_quest_mods_masterlist_2021/
Also check out endless/random encounters mods like The Endless Pit, The Rabbit Hole, Forgotten Dungeons, The Hidden City, Radiance, Arena and Immersive World Encounters - they make the game feel more random and exciting.