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The longer you wait, the more out leveled you'll be for the content so won't get much exp clearing it if you finish the rest of normal content first. Personally I thought Atlantis difficulty felt a bit spiky at times, so may be easier to do Act 4 first then Atlantis then Act 5 but you can also try doing Atlantis first and if you find it too difficult, swap back to Act 4.
enemy level-wise : same as act IV
However, sometimes I like to do it before act 4 especially if I don't have enough vitality resistance.
Lore wise you could also argue to do it after arriving back in Korinth but before meeting the quest NPC to head north.