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However you could use blender to model your scene, mimic some of the material properties and use the freestyle line renderer to create an overlay for the edges.
It is possible to do that using a combination of blender for 3d and tools like photoshop and gimp, or even the blender compositor to make the color effect happen.
If you are really good at drawing you could also use blenders 2d animation tools and simply draw the stuff and animate it the traditional way.
However in terms of image editors/ painting tools the options are plenty. Gimp, Krita, Mypaint etc. all do the trick if you know what you are going for.
Gimp is free and might let you achieve that look. Alongside a tablet so you can hand draw stuff, you can get a reasonable starter tablet for around 50 bucks.