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To answer your question though, I'd recommend watching Seasons 1 - 5 all the way to see the spies' missions from high school to college since they're college students in the new season (and this game), just going to a different school in Singapore. I think the first 2 seasons best encapsulate the silliness of the show, and Seasons 3 - 4 have some special episodes, such as the 3-part season finale "Evil Promotion" in S3.
You could also start with the Totally Spies Movie, which serves as the prequel for the show telling the story of how the girls started working for WOOHP, but I will warn you - that movie is inconsistent with the show AF, idk what they were thinking. It's basically a prolonged (Season 6) episode to fit a movie length, but it isn't the show's best story. I'd recommend watching the series since their origin is explained in later episodes anyway.
oh, and you can skip season 6
Here's the playlist for Season 1