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It might heavily depend on the driver version used and it might depend on the desktop environment and kernel used. Forget distributions.
Both Unity and KDE do unredirect fullscreen windows so there isn't much off a difference. Also why would you want to switch the distro just to get a different desktop. That makes no sense.
Anywho: make sure that what's causing the performance-problem isn't the CPU switching between frequencies because of the Ondemand-profile.
A quick fix for this:
sudo apt-get install cpufrequtils
cpufreq-info
(this will fail if there is no governor running)
If there are no errors reported and cpufreq-info reports a governor running, change it with
sudo cpufreq-set -g performance
and report back.
It is available in the repositories of some distros, a ppa for ubuntu and of course also as source code.
On openSUSE 12.3 64 bit the Catalyst 13.8 works great.
It solved all performance issues, I had with Serious Sam 3.
Left for Dead 2 runs better too then before.
HD5750 1 gig of ram.
You can try openSUSE, but I would make sure first, the instalation of the catalyst drivers is not just messed up. Because that is most lickely your problem.
Linux is all about choice, but every distro uses about the same kernel.
One more thing about openSUSE, it has a one clcik install for the Catalsyst drivers, but not for the beta versions.
So to install beta drivers on openSUSE, you need the commandline.
Did you try what Wouter sugested ?