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You can increase the amount of Smite Buildup you do by adding salts, Radiant weapon spell, and others into the mix. I (for example) use Flickering Flail, 3x Satus runes, Radiant Weapon spell, maxed Exacter Scripture, and amu + rings that increase spellpower (which does make all spells hit harder/heal more!) This will contribute to how much more Smite Buildup you make in enemies (minus their resistance to the damage type of course)
TL;DR
Radiant Damage is just a Damage type (like Fire, Inferno, etc.); Smite Buildup is its Status effect. More Radiant in build, faster build of Smite (and possibly more damage when it procs).