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Also check Cass, she sells them from time to time.
Let me explain the system.
If you only have 1 pistol, 1 long gun etc at 15+ the game will give you a lot of hardened iron.
If you have a lot of lower level gear the game will give you a lot of lower tier materials too instead and you get way less hardened iron.
But you do not need +20 weapons for the final fight, i started getting hardened once i started playing nightmare adventure after the story ended.
Your gear score also influences drops. At 20, you will get only hardened and very rarely low tier ones.
they drop from every area, its just not super common as they share the same pool as iron, forged iron and galvanized iron too and it also depends on your overall power level
That seems insanely wrong, BOTH of my guns are 15, they were when I went into the RE, NO hardened have dropped except once.
Do you have guns in your inventory that are not near 15? Is your power level 16-17 at least?